Don't really know if that's possible unless you actually take one of the tanks apart and then silicone it how you want it. Don't recommend doing this though. What size are the tanks? Just get something like a 29 gal and then convert it to a tall.
I have a waterfall in mine but I don't even run it. Only thing it does it add a bit of humidity and the rest is just for looks. Pump issues are usually a problem and depending how you set up your false bottom it can be hard to do pump maintenance.
Regardless if you wanted a waterfall you would still need to have something that the frog can soak in, so the pond would be good. And I clean my tank about once a week, taking all the plants, water bowl, vines out and then rinsing them all with treated water. Make sure you use treated water as tap water is bad for them. Also only use distilled/reverse osmosis water for misting. Let me know if there is anything else you need and I will try to help.





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